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材料工程  2018, Vol. 46 Issue (5): 11-21    DOI: 10.11868/j.issn.1001-4381.2017.000440
  石墨烯专栏 本期目录 | 过刊浏览 | 高级检索 |
氧化石墨烯复合材料吸附铀的研究进展
刘红娟1, 谢水波2,3, 张希晨3, 刘迎九3, 曾涛涛3
1. 南华大学 核科学技术学院, 湖南 衡阳 421001;
2. 南华大学 铀矿冶生物技术国防重点学科实验室, 湖南 衡阳 421001;
3. 南华大学 污染控制与资源化技术湖南省重点实验室, 湖南 衡阳 421001
Research Progress of Graphene Oxide Composite Materials for Uranium Adsorption
LIU Hong-juan1, XIE Shui-bo2,3, ZHANG Xi-chen3, LIU Ying-jiu3, ZENG Tao-tao3
1. Institute of Nuclear Science and Technology, University of South China, Hengyang 421001, Hunan, China;
2. Key Discipline Laboratory for National Defence for Biotechnology in Uranium Mining and Hydrometallurgy, University of South China, Hengyang 421001, Hunan, China;
3. Hunan Province Key Laboratory of Pollution Control and Resources Reuse Technology, University of South China, Hengyang 421001, Hunan, China
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摘要 氧化石墨烯由于具有超大的比表面积、高强度和化学稳定性好等优点,其在环保领域作为含铀废水吸附材料的应用潜能备受关注。本文综述了近年来石墨烯基复合材料吸附水溶液中铀的研究现状及进展,介绍了石墨烯基复合材料对铀的吸附性能,分析了溶液pH值、温度、离子强度、接触时间和吸附剂用量等因素对吸附效果影响的原理,阐述了通过表面络合模型,光谱分析和理论计算等方法探讨氧化石墨烯复合材料的微观形貌结构与铀吸附效果之间的内在联系,最后研究了氧化石墨烯复合材料吸附铀研究中面临的挑战,对石墨烯材料与轴的相互作用机理及其在环保方面的开发应用进行了展望。
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刘红娟
谢水波
张希晨
刘迎九
曾涛涛
关键词 石墨烯复合材料吸附微观结构    
Abstract:Graphene oxide has potential application prospects in the field of environmental protection as the adsorption material of uranium-containing wastewater due to its many advantages such as its large specific surface area, high mechanical strength and good chemical stability, which has attracted much attention. The research situation and progress of uranium adsorption of graphene-oxide composite materials were summarized in this paper. The principle about effect of solution pH value, temperature, ionic strength, contact time and adsorbent dosage on uranium adsorption by graphene oxide composite materials was analyzed. The study on internal relationship between the microstructure and micromorphology of graphene oxide composite materials and uranium adsorption capacity by the methods of surface complexation model, spectral analysis and theoretical calculation was elaborated. Meanwhile, the challenges in the study of the adsorption of uranium by graphene oxide composite materials were studied, the research on the interaction mechanism of uranium and graphene oxide materials and their development and application in environmental protection were prospected.
Key wordsgraphene    composite material    uranium    adsorption    microstructure
收稿日期: 2017-04-11      出版日期: 2018-05-16
中图分类号:  O613.71  
  TB33  
通讯作者: 谢水波(1964-),男,教授,博士研究生导师,主要从事新型吸附材料在核环境治理与修复的研究,联系地址:湖南省衡阳市南华大学铀矿冶生物技术国防重点学科实验室(421001),E-mail:xiesbmr@263.net     E-mail: xiesbmr@263.net
引用本文:   
刘红娟, 谢水波, 张希晨, 刘迎九, 曾涛涛. 氧化石墨烯复合材料吸附铀的研究进展[J]. 材料工程, 2018, 46(5): 11-21.
LIU Hong-juan, XIE Shui-bo, ZHANG Xi-chen, LIU Ying-jiu, ZENG Tao-tao. Research Progress of Graphene Oxide Composite Materials for Uranium Adsorption. Journal of Materials Engineering, 2018, 46(5): 11-21.
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http://jme.biam.ac.cn/CN/10.11868/j.issn.1001-4381.2017.000440      或      http://jme.biam.ac.cn/CN/Y2018/V46/I5/11
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